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1、题目：Methane from synthesis gas and operation of high-temperature methanation
类型Original Research Article
刊物：Nuclear Engineering and Design, Volume 78, Issue 2, 1 April 1984,
Pages 241-250
作者：B. Höhlein, H. Niessen, J. Range, H.J.R. Schiebahn, M. Vorwerk
2、题目：The Effect Of Preparation Method Upon The Structures, Stability And Metal/Support Interactions In Nickel/Alumina Catalysts
类型：Original Research Article
刊物：Studies in Surface Science and Catalysis, Volume 16, 1983, Pages 237-
271
作者：D.C. Puxley, I.J. Kitchener, C. Komodromos, N.D. Parkyns
3、题目：Catalyst design for reactions with synthesis gas
类型：Original Research Article
刊物：Studies in Surface Science and Catalysis, Volume 133, 2001, Pages 399-407
作者：G.P. Valença, E.S. Gonçalves
4、题目：Production of Methanation Catalysts
类型：Original Research Article
刊物：Studies in Surface Science and Catalysis, Volume 1, 1976, Pages 331-
341
作者：George W. Bridger, Colin Woodward
5、题目：The Design and Testing of A New Range of Methanation Catalysts
类型：Original Research Article
刊物：Studies in Surface Science and Catalysis, Volume 7, Part 1, 1981, Pages
517-528
作者：D.L. Trimm, E.R. Karal
6、题目：Deactivation Phenomena of a Ni-based Catalyst for High Temperature Methanation
类型：Original Research Article
刊物：Studies in Surface Science and Catalysis, Volume 6, 1980, Pages 459-469
作者：H.H. Gierlich, M. Fremery, A. Skov, J.R. Rostrup-Nielsen

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关键词：elsevier 英文文献 vier else LSE 文献 英文 elsevier

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6 全文看不了.
  Studies in Surface Science and Catalysis
  Volume 6, 1980,Pages 459-469
Catalyst Deactivation  

doi:10.1016/S0167-2991(08)65253-2 | How to Cite or Link Using DOI Copyright © 1980 Elsevier Scientific Publishing Company Published by Elsevier B.V.

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Deactivation Phenomena of a Ni-based Catalyst for High Temperature Methanation


This article is not included in your organization's subscription. However, you may be able to access this article under your organization's agreement with Elsevier.



H.H. Gierlich1, M. Fremery2, A. Skov2 and J.R. Rostrup-Nielsen2


Available online 1 January 2009.  

The deactivation phenomena of a Ni-based catalyst for high temperature methanation were investigated in pilot plant experiments under industrial conditions. The mechanism of catalyst deactivation by encapsulating carbon formation (β-deactivation) and the influence of sulphur are discussed. Ways of suppressing β-deactivation are demonstrated.





















1 Union Rheinische Braunkohlen Kraftstoff AG, Wesseling

2 Haldor Topsøe A/S, Copenhagen

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4.也没全文:(
  Studies in Surface Science and Catalysis
  Volume 133, 2001,Pages 399-407
Reaction Kinetics and the Development and Operation of Catalytic Processes, Proceedings of the 3rd International Symposium  

doi:10.1016/S0167-2991(01)81988-1 | How to Cite or Link Using DOI Copyright © 2001 Elsevier B.V. All rights reserved.

Permissions & Reprints

Catalyst design for reactions with synthesis gas


This article is not included in your organization's subscription. However, you may be able to access this article under your organization's agreement with Elsevier.



G.P. Valença, a and E.S. Gonçalvesa

aDepartment of Chemical Processes, School of Chemical Engineering, CampinasState University, UNICAMP, 13081-970, Campinas, SP, Brazil



Available online 8 August 2007.  

Bond Order Conservation-Morse Potential (BOC-MP) formalism is used tostudy the change in activation energy for different elementary steps involving all possible chemical species on any metallic surface in order to identify optimum catalysts for the production of methane, methanol or ethylene from synthesis gas. All possible steps are analyzed for the methanation reaction. It is assumed that the reaction occurs on pure metallic surfaces, thus, the influence of the support or promoters is not taken into account. The method suggests that Ni is a more selective for methanation reaction, in agreement with the fact that Ni/Si02 is the real catalyst used industrially. On the other hand on the surface of Fe or W the reaction may result in the formation of adsorbed C, also in agreement with experiment.